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The features of birefringence of the linearly polarized light in the magnetoelectric single crystals LiNiPO4 |
Yura Kharchenko |
Institute for Low Temperature Physics, 47 Lenin ave., Kharkov 61103, Ukraine |
Abstract |
The magnetization of the antiferromagnetic magnetoelectric LiNiPO4 single crystal along the crystallographic axes a, b and c was measured. The carried out researches have shown in it presence of a weak ferromagnetism. The weak ferromagnetic moment is directed along the antiferromagnetic axis of the crystal. The measured remanent magnetization in LiNiPO4 is equal to about 0.005 G at 5K. With increase of a temperature of the sample up to the Neel temperature (TN~21K) the remanent magnetic moment was decreasing up to zero. Furthermore, in LiNiPO4 the intermediate antiferromagnetic phase was revealed in the narrow temperature interval ~1 K near Neel temperature. The magnetic structure of the basic antiferromagnetic state of LiNiPO4 is uniform, but its antiferromagnetic intermediate state has a modulated structure. For more information about processes of magnetic ordering the behaviour of birefringence in this crystal was investigated depending on changes of temperature or intensity of a magnetic field. So, on the temperature dependences of birefringence is observed jump at Т1 and at Т2 (=Т1+1К) break of a curve. These features to make agree with presence intermediate of structure in a temperature interval Т1-Т2. But herewith the temperature hysteresis with width 6 K and the centre in the TN is observed. In addition, we notice linear dependence of birefringence on intensity of a magnetic field in fields up to 15 kOe and further break of a curve. In higher magnetic fields, the dependence carries parabolic character. The attempt is made to connect these features with behaviour of magnetic structure in a magnetic field. (ilt.kharkov.ua/bvi/structure/depart_e/d04/resecher-en.html) |
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Presentation: Poster at E-MRS Fall Meeting 2006, Symposium I, by Yura KharchenkoSee On-line Journal of E-MRS Fall Meeting 2006 Submitted: 2006-05-13 17:04 Revised: 2009-06-07 00:44 |