Design and synthesis of organic molecules possessing significant second harmonic generation response is of great interest owing to their versatile applications in the field of existing and future technologies. Organic materials are always preferred in material science due to their easy tailoring and high solubility over pure inorganic materials. A series of small chiral phthalimides have been designed and synthesized with the aim to explore their structural features and their nonlinear optical properties. The composition of newly prepared molecules was confirmed by analytical and spectroscopic techniques and also by single crystal X-ray diffraction technique. The interesting and enthusing results are observed and will be presented. 

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