Yb³⁺-doped Bi₄Si₃O₁₂ single crystals with good optical quality have been grown by the modified vertical Bridgman method. The crystalline quality of the Yb³⁺: Bi₄Si₃O₁₂ single crystal was verified by the width of the X-ray diffraction (XRD) peak in the X-ray rocking curves measurement. The absorption spectrum and emission spectra and fluorescence lifetime of the Yb³⁺: Bi₄Si₃O₁₂ crystal were detected at room temperature. The spectral and laser parameters of Yb³⁺: Bi₄Si₃O₁₂ crystal have been calculated.

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